To address this specific gap, Vanadium Redox Flow Batteries (VRFBs) have emerged as a powerful and promising technology tailored for large-scale energy storage , . The defining characteristic of a VRFB is the unique decoupling of its power and energy capacity.
Crossover provides an internal short-circuit path, causing the CE to be less than 100 % . Understanding the mechanistic basis and consequences of vanadium ion crossover is essential for rational membrane design, performance prediction, and the long-term viability of large-scale VRFB systems.
During operation, all four species cross the membrane in both directions, but the net flux is unbalanced. The total amount of vanadium crossing from the negative half-cell (as V 2+ and V 3+) is typically greater than the amount crossing from the positive half-cell (as VO 2+ and VO 2+) .
The mechanism unfolds through a sequence of events: As established, the permeability of vanadium ions through a typical CEM follows the order V 2+ > VO 2+ > VO 2+ > V 3+ . During operation, all four species cross the membrane in both directions, but the net flux is unbalanced.
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